Structural Change of the Mn Cluster during the S2→S3 State Transition of the Oxygen-Evolving Complex of Photosystem II. Does It Reflect the Onset of Water/Substrate Oxidation? Determination by Mn X-ray Absorption Spectroscopy.

Structural Change of the Mn Cluster during the S2→S3 State Transition of the Oxygen-Evolving Complex of Photosystem II. Does It Reflect the Onset of Water/Substrate Oxidation? Determination by Mn X-ray Absorption Spectroscopy.

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Structural changes in the Mn4Ca cluster and the mechanism of photosynthetic water splitting Mn4Ca cluster in photosynthesis: where and how water is oxidized to dioxygen X-ray spectroscopy-based structure of the Mn cluster and mechanism of photosynthetic oxygen evolution Mn K-edge XANES and Kbeta XES studies of two Mn-oxo binuclear complexes: investigation of three different oxidation states relevant to the oxygen-evolving complex of photosystem II Focusing the view on nature's water-splitting catalyst.Activation of a water molecule using a mononuclear Mn complex: from Mn-aquo, to Mn-hydroxo, to Mn-oxyl via charge compensation.The first room-temperature X-ray absorption spectra of higher oxidation states of the tetra-manganese complex of photosystem II.Calcium ligation in photosystem II under inhibiting conditions.Kinetic modeling of the X-ray-induced damage to a metalloprotein.Calcium exchange and structural changes during the photosynthetic oxygen evolving cycle.Calcium in the oxygen-evolving complex: structural and mechanistic role determined by X-ray spectroscopy.Light-dependent production of dioxygen in photosynthesis.The water-oxidation complex in photosynthesis.X-ray spectroscopy of the Mn4Ca cluster in the water-oxidation complex of Photosystem II.Computational studies of the O(2)-evolving complex of photosystem II and biomimetic oxomanganese complexes Oxidation state changes of the Mn4Ca cluster in photosystem II.Computational insights into the O2-evolving complex of photosystem II.An intrinsically disordered photosystem II subunit, PsbO, provides a structural template and a sensor of the hydrogen-bonding network in photosynthetic water oxidation.Structural changes of the oxygen-evolving complex in photosystem II during the catalytic cycle.Where water is oxidized to dioxygen: structure of the photosynthetic Mn4Ca cluster from X-ray spectroscopy The Mn cluster in the S(0) state of the oxygen-evolving complex of photosystem II studied by EXAFS spectroscopy: are there three Di-mu-oxo-bridged Mn(2) moieties in the tetranuclear Mn complex?FTIR spectra and normal-mode analysis of a tetranuclear manganese adamantane-like complex in two electrochemically prepared oxidation states: relevance to the oxygen-evolving complex of photosystem II Absence of Mn-centered oxidation in the S(2) --> S(3) transition: implications for the mechanism of photosynthetic water oxidation.Why nature chose Mn for the water oxidase in Photosystem II.Rationalizing the 2.25 Å Resolution Crystal Structure of the Water Oxidising Complex of Photosystem II in the S3 State.Structural Changes Correlated with Magnetic Spin State Isomorphism in the S2 State of the Mn4CaO5 Cluster in the Oxygen-Evolving Complex of Photosystem II.Is Mn-Bound Substrate Water Protonated in the S(2) State of Photosystem II?The interaction of His337 with the Mn4Ca cluster of photosystem II.Structural changes of D1 C-terminal alpha-carboxylate during S-state cycling in photosynthetic oxygen evolution.Metal oxidation states in biological water splitting† †Electronic supplementary information (ESI) available: Additional methodological details and discussion, Tables S1–S10, Fig. S1–S16, spin populations, parameters of optimized structures, experime Metal oxidation states in biological water splitting.

P2860

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P2860

Structural Change of the Mn Cluster during the S2→S3 State Transition of the Oxygen-Evolving Complex of Photosystem II. Does It Reflect the Onset of Water/Substrate Oxidation? Determination by Mn X-ray Absorption Spectroscopy.

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