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Enantioselective construction of remote quaternary stereocentres

Enantioselective construction of remote quaternary stereocentres

http://www.wikidata.org/entity/Q33554259

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Remote carboxylation of halogenated aliphatic hydrocarbons with carbon dioxide.Palladium-Catalyzed Enantioselective Heck Alkenylation of Trisubstituted Allylic Alkenols: A Redox-Relay Strategy to Construct Vicinal Stereocenters Coupling of sterically hindered trisubstituted olefins and benzocyclobutenones by C-C activation: total synthesis and structural revision of cycloinumakiol.Investigating the nature of palladium chain-walking in the enantioselective redox-relay Heck reaction of alkenyl alcohols Synthesis of highly functionalized tri- and tetrasubstituted alkenes via Pd-catalyzed 1,2-hydrovinylation of terminal 1,3-dienes.Development and Investigation of a Site Selective Palladium-Catalyzed 1,4-Difunctionalization of Isoprene using Pyridine-Oxazoline Ligands.Palladium-Catalyzed Cross-Coupling of α-Bromocarbonyls and Allylic Alcohols for the Synthesis of α-Aryl Dicarbonyl Compounds.ORGANIC CHEMISTRY. Catalytic asymmetric hydroamination of unactivated internal olefins to aliphatic amines Enantioselective and Regiodivergent Copper-Catalyzed Electrophilic Arylation of Allylic Amides with Diaryliodonium Salts Relative reactivity of alkenyl alcohols in the palladium-catalyzed redox-relay Heck reaction.Palladium-catalyzed enantioselective 1,1-fluoroarylation of aminoalkenes.Rh-Catalyzed Desymmetrization of α-Quaternary Centers by Isomerization-Hydroacylation.Catalytic enantioselective synthesis of quaternary carbon stereocentres A direct approach to amines with remote stereocentres by enantioselective CuH-catalysed reductive relay hydroamination Alkenyl carbonyl derivatives in enantioselective redox relay Heck reactions: accessing α,β-unsaturated systems Palladium-catalyzed enantioselective Heck alkenylation of acyclic alkenols using a redox-relay strategy.Enantioselective Dehydrogenative Heck Arylations of Trisubstituted Alkenes with Indoles to Construct Quaternary Stereocenters Enantioselective Palladium-Catalyzed Alkenylation of Trisubstituted Alkenols To Form Allylic Quaternary Centers.Enantioselective oxidative boron Heck reactions.Remote functionalization through alkene isomerization.Ligand-Controlled Regiodivergent Copper-Catalyzed Alkylboration of Alkenes.Formation of C(sp(3) )-C(sp(3) ) Bonds through Nickel-Catalyzed Decarboxylative Olefin Hydroalkylation Reactions.Nickel-catalyzed synthesis of 1,1-diborylalkanes from terminal alkenes.Palladium-Catalyzed Enantioselective Redox-Relay Heck Alkynylation of Alkenols To Access Propargylic Stereocenters.Stereospecific Cross Couplings To Set Benzylic, All-Carbon Quaternary Stereocenters in High Enantiopurity.Diazafluorenone-Promoted Oxidation Catalysis: Insights into the Role of Bidentate Ligands in Pd-Catalyzed Aerobic Aza-Wacker Reactions.Palladium-Catalyzed Enantioselective Redox-Relay Heck Arylation of 1,1-Disubstituted Homoallylic Alcohols.Introducing unactivated acyclic internal aliphatic olefins into a cobalt catalyzed allylic selective dehydrogenative Heck reaction Chain Walking of Allylrhodium Species Towards Esters During Rhodium-Catalyzed Nucleophilic Allylations of Imines The development and mechanistic investigation of a palladium-catalyzed 1,3-arylfluorination of chromenes.A unique Pd-catalysed Heck arylation as a remote trigger for cyclopropane selective ring-opening Zirconocene-assisted remote cleavage of C-C and C-O bonds: application to acyclic stereodefined metalated hydrocarbons.Enantioselective Construction of Acyclic Quaternary Carbon Stereocenters: Palladium-Catalyzed Decarboxylative Allylic Alkylation of Fully Substituted Amide Enolates.Access to enantioenriched 2,3- and 2,5-dihydrofurans with a fully substituted C2 stereocenter by Pd-catalyzed asymmetric intermolecular Heck reaction.Stereodefined acyclic trisubstituted metal enolates towards the asymmetric formation of quaternary carbon stereocentres.Remote functionalization of hydrocarbons with reversibility enhanced stereocontrol.Palladium-Catalyzed Enantioselective Narasaka-Heck Reaction/Direct C-H Alkylation of Arenes: Iminoarylation of Alkenes.Enabling the Cross-Coupling of Tertiary Organoboron Nucleophiles through Radical-Mediated Alkyl Transfer.Diastereoselective Synthesis of Highly Substituted Tetrahydrofurans by Pd-Catalyzed Tandem Oxidative Cyclization-Redox Relay Reactions Controlled by Intramolecular Hydrogen Bonding.Terminal-Selective Functionalization of Alkyl Chains by Regioconvergent Cross-Coupling.

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Enantioselective construction of remote quaternary stereocentres

http://www.wikidata.org/entity/Q33554259

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2014 nî lūn-bûn

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2014 թուականի Ապրիլին հրատարակուած գիտական յօդուած

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2014 թվականի ապրիլին հրատարակված գիտական հոդված

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2014年の論文

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2014年論文

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2014年論文

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2014年論文

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2014年論文

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2014年論文

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2014年论文

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres.

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres.

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres

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Enantioselective construction of remote quaternary stereocentres.

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Enantioselective construction of remote quaternary stereocentres

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Harshkumar H Patel

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Matthew S Sigman

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Tian-Sheng Mei

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P2860

Asymmetric intermolecular boron Heck-type reactions via oxidative palladium(II) catalysis with chiral tridentate NHC-amidate-alkoxide ligands

The heck reaction as a sharpening stone of palladium catalysis.

The asymmetric Heck and related reactions.

Enantio- and diastereodivergent dual catalysis: α-allylation of branched aldehydes.

A highly selective and general palladium catalyst for the oxidative Heck reaction of electronically nonbiased olefins.

Palladium-catalyzed asymmetric conjugate addition of arylboronic acids to five-, six-, and seven-membered β-substituted cyclic enones: enantioselective construction of all-carbon quaternary stereocenters.

Imparting catalyst control upon classical palladium-catalyzed alkenyl C-H bond functionalization reactions

Enantioselective redox-relay oxidative heck arylations of acyclic alkenyl alcohols using boronic acids.

Oxidative palladium(II) catalysis: A highly efficient and chemoselective cross-coupling method for carbon-carbon bond formation under base-free and nitrogenous-ligand conditions

Catalytic asymmetric synthesis of all-carbon quaternary stereocenters

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340-344

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scholarly article

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10.1038/NATURE13231

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7496

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508

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1001746296

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24717439

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enantioselectivity

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4007023

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