Structure of Estradiol Metal Chelate and Estrogen Receptor Complex: The Basis for Designing a New Class of Selective Estrogen Receptor ModulatorsA novel liquid organic hydrogen carrier system based on catalytic peptide formation and hydrogenation.Aromatic vs aliphatic C-H bond activation by rhodium(I) as a function of agostic interactions: catalytic H/D exchange between olefins and methanol or water.Nucleophilic de-coordination and electrophilic regeneration of "hemilabile" pincer-type complexes: formation of anionic dialkyl, diaryl, and dihydride Pt(II) complexes bearing no stabilizing pi-acceptors.Cationic, neutral, and anionic PNP Pd(II) and Pt(II) complexes: dearomatization by deprotonation and double-deprotonation of pincer systems.DFT study of the structure and reactivity of the terminal Pt(IV)-oxo complex bearing no electron-withdrawing ligands.Direct synthesis of amides from alcohols and amines with liberation of H2.In vivo magnetic resonance imaging of the estrogen receptor in an orthotopic model of human breast cancer.Direct Synthesis of Symmetrical Azines from Alcohols and Hydrazine Catalyzed by a Ruthenium Pincer Complex: Effect of Hydrogen BondingApplications of acceptorless dehydrogenation and related transformations in chemical synthesis.Metal-ligand cooperation.Hydrogenation and Hydrosilylation of Nitrous Oxide Homogeneously Catalyzed by a Metal Complex.The Ferraquinone-Ferrahydroquinone Couple: Combining Quinonic and Metal-Based Reactivity."Long-range" metal-ligand cooperation in H2 activation and ammonia-promoted hydride transfer with a ruthenium-acridine pincer complex.Effect of CO on the oxidative addition of arene C-H bonds by cationic rhodium complexes.Metal-ligand cooperation in the trans addition of dihydrogen to a pincer Ir(I) complex: a DFT study.Direct deamination of primary amines by water to produce alcohols.Oxidative addition of water to novel Ir(I) complexes stabilized by dimethyl sulfoxide ligands.The first fully characterized neutral and cationic rhodium(I)-complexes containing DMSO as the only dative ligand; S-, O- and bridging S,O-bidentate binding modes.Oxidative addition of water and aliphatic alcohols by IrCl(trialkylphosphine)(3).Ru(0) and Ru(II) nitrosyl pincer complexes: structure, reactivity, and catalytic activity.Selective ortho C-h activation of haloarenes by an Ir(I) system.Novel azine reactivity: facile N-N bond cleavage, C-H activation, and N-N coupling mediated by RhI.A new ligand system based on a bipyridine-functionalized calix[4]arene backbone leading to mono- and bimetallic complexes.Direct synthesis of pyrroles by dehydrogenative coupling of β-aminoalcohols with secondary alcohols catalyzed by ruthenium pincer complexes.Metallacarbenes from diazoalkanes: an experimental and computational study of the reaction mechanism.Interplay between solvent and counteranion stabilization of highly unsaturated rhodium(III) complexes: facile unsaturation-induced dearomatization.C-C versus C-H activation and versus agostic C-C interaction controlled by electron density at the metal center.Dimethylsulfoxide as a ligand for RhI and IrI complexes--isolation, structure, and reactivity towards X-H bonds (X=H, OH, OCH3).Metal-stabilized phenoxonium cation.New ligand systems incorporating two and three 4,4'-bipyridine units. Characterization of bi- and trimetallic rhodium and iridium complexes.Self-oxidation of a phenolate complex to a bimetallic stilbene quinone.Pi-accepting-pincer rhodium complexes: an unusual coordination mode of PCP-type systems.Formal loss of an H radical by a cobalt complex via metal-ligand cooperation.Direct conversion of alcohols to acetals and H(2) catalyzed by an acridine-based ruthenium pincer complex.Iron pincer complex catalyzed, environmentally benign, E-selective semi-hydrogenation of alkynes.Activation of nitriles by metal ligand cooperation. Reversible formation of ketimido- and enamido-rhenium PNP pincer complexes and relevance to catalytic design.Competitive C-I versus C-CN reductive elimination from a Rh(III) complex. Selectivity is controlled by the solvent.Reactivity of rhodium-triflate complexes with diphenylsilane: evidence for silylene intermediacy in stoichiometric and catalytic reactions.Pyridine-based SNS-iridium and -rhodium sulfide complexes, including d8-d8 metal-metal interactions in the solid state.
P50
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P50
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Duits scheikundige
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David Milstein
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David Milstein
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